Berryville is a city in Carroll County, Arkansas, United States. The population was 5,682 at the 2020 census. making it the largest city in Carroll County. Along with Eureka Springs, it is one of the two county seats of Carroll County.

Carroll County is a county located in the U.S. state of Arkansas. As of the 2020 census, the population was 28,260. The county has two county seats, Berryville and Eureka Springs. Carroll County is Arkansas's 26th county, formed on November 1, 1833, and named after Charles Carroll, the last surviving signer of the United States Declaration of Independence.