Pomfret is a town located in Windham County, Connecticut with a population of 4,266 according to the 2020 United States Census. The town is part of the Northeastern Connecticut Planning Region. The town was incorporated in 1713 and was named after Pontefract in West Yorkshire, England. The land on which Pomfret stands today was purchased from Native Americans in 1686 in a deal known as the "Mashmuket Purchase" or "Mashamoquet Purchase".

Windham County is one of the eight historical counties in the U.S. state of Connecticut, located in its northeastern corner. As of the 2020 census, the population was 116,418, making it the least populous county in Connecticut. It forms the core of the region known as the Quiet Corner. Windham County is included in the Worcester, MA-CT Metropolitan Statistical Area, which is also included in the Boston-Worcester-Providence, MA-RI-NH-CT Combined Statistical Area. The entire county is within the Quinebaug and Shetucket Rivers Valley National Heritage Corridor, as designated by the National Park Service.